Response: Atrazine Profile

Gabriel A. Hegyes (GHEGYES@CSRS.ESUSDA.GOV)
Thu, 03 Nov 1994 15:05:13 -0500 (EST)

E X T O X N E T

EXTENSION TOXICOLOGY NETWORK

A Pesticide Information Project of Cooperative Extension Offices

of Cornell University, Michigan State University, Oregon State

University, and University of California at Davis. Major support

and funding was provided by the USDA/Extension Service/National

Agricultural Pesticide Impact Assessment Program.

Revised 9/93.

EXTOXNET primary files maintained and archived at Oregon State

University.

Atrazine

TRADE OR OTHER NAMES

G-30027, Aatrex, Aktikon, Alazine, Atred, Atranex, Atrataf,

Atratol, Azinotox, Crisazina, Farmco Atrazine, Gesaprim, Giffex

4L, Malermais, Primatol, Simazat, Zeaphos (25).

REGULATORY STATUS

Atrazine has been classified as a Restricted Use Pesticide

(RUP), due to its potential for groundwater contamination (32).

RUPs may be purchased and used only by certified applicators.

Products containing atra-zine must bear the signal word "Caution"

(25).

INTRODUCTION

Atrazine is a selective triazine herbicide used to control

broadleaf and grassy weeds in corn, sorghum, sugarcane,

pineapple, Christmas trees and other crops, and in conifer

reforestation plantings. It is also used as a non-selective

herbicide on non-cropped industrial lands and on fallow lands.

It is available as dry flowable, flowable liquid, liquid, water

dispersible granular, and wettable powder formulations (25, 28).

TOXICOLOGICAL EFFECTS

ACUTE TOXICITY

Atrazine is slightly to moderately toxic to humans and other

animals. It can be absorbed into the bloodstream through oral,

dermal and inhalation exposure. Symptoms of poisoning include

abdominal pain, diarrhea and vomiting, eye irritation, irritation

of mucous membranes, and possible skin reactions (14). At very

high doses, rats showed excitation followed by depression, slowed

breathing, incoordination, muscle spasms, and hypothermia (24).

After consuming a large oral dose, rats exhibited muscular

weakness, hypoactivity, breathing difficulty, prostration,

convulsions and death (33).

Atrazine is a mild skin irritant. Rashes associated with

exposure have been reported. Moderate to severe eye irritation

can occur. Exposure to large concentrations of airborne

particles or droplets may cause irritation of the mucous

membranes (24, 30).

The amount of atrazine that is lethal to one-half (50%) of

experimental animals fed the material is referred to as its acute

oral lethal dose fifty, or LD50. The oral LD50 for atrazine in

rats is 672 to 3,000 mg/kg, in mice is 850 to 1,750 mg/kg, in

rabbits is 750 mg/kg, and in hamsters is 1,000 mg/kg. The dermal

LD50 in rabbits is 7,500 mg/kg, and in rats is greater than 3,000

mg/kg.

The lethal concentration fifty, or LC50, is that

concentration of a chemical in air or water that kills half of

the experimental animals exposed to it for a set time period.

The one-hour inhalation LC50 in rats is greater than 700 mg/m3.

The 4-hour inhalation LC50 in rats is 5,200 mg/m3 (24, 25, 33,

NIOSH RTECS Online File # 85/8408).

CHRONIC TOXICITY

Forty percent of rats receiving oral doses of 20 mg/kg/day

for 6 months died with signs of respiratory distress and

paralysis of the limbs. Morphological and biochemical changes in

the brain, heart, liver, lungs, kidney, ovaries and endocrine

organs were observed (30). Rats fed 5 or 25 mg/kg/day of

atrazine for 6 months exhibited growth retardation. Examination

of these rats revealed no lesions (24). In a 2-year study with

dogs fed 0, 0.75. 7.5 or 75 mg/kg/day, the NOAEL was 0.75 mg/kg.

At 7.5 mg/kg, decreased food intake and increased heart and liver

weights were observed. At 75 mg/kg, there were decreases in food

intake and body weight gain, increased adrenal weight, lowered

blood cell counts, and occasional tremors or stiffness in the

rear limbs (29).

The EPA has established a Lifetime Health Advisory level for

atrazine in drinking water of 3 micrograms per liter (ug/l).

Water containing atrazine at or below this level is acceptable

for drinking every day over the course of one's lifetime, and

does not pose any health risk. Long-term consumption of high

levels of atrazine has caused adverse health effects in animals,

including tremors, changes in organ weights and damage to the

liver and heart (29).

Reproductive Effects

Subcutaneous injection of atrazine of near lethal doses of

800 mg/kg/day on days 3, 6 and 9 of gestation resulted in the

death and resorption of some or all the pups in each litter of

rats. Dosages as high as 200 mg/kg/day by this route did not

affect the number of pups per litter or their weight at weaning.

Dietary levels up to 1,000 ppm (about 50 mg/kg/day) caused no

adverse effects (24).

Teratogenic Effects

In mice, atrazine did not cause abnormalities in fetuses

whose dams were given doses of 46.4 mg/kg/day during days 6

through 14 of gestation (24).

Mutagenic Effects

The weight of evidence from more than 50 studies reported in

the literature indicates that atrazine is not mutagenic (24). In

tests with mice, atrazine induced dominant lethal mutations and

increased the frequency of chromatid breaks in bone marrow (29).

Carcinogenic Effects

Atrazine did not cause tumors when mice were given oral

doses of 21.5 mg/kg/day from age 1 to 4 weeks followed by dietary

doses of 82 mg/kg for an additional 17 months. Mammary tumors

were observed in rats after lifetime administration of atrazine

(24). EPA has classified atrazine as a possible human carcinogen

because it has caused cancer in rats receiving high doses over

the course of their lifetimes (29).

Organ Toxicity

Lethal doses in test animals have caused severe damage, in

the form of congestion and/or hemorrhaging, to the lungs,

kidneys, liver, spleen, brain and heart (29).

Fate in Humans and Animals

Ingested atrazine is readily absorbed into the body through

the gastrointestinal tract. When a single dose of 0.53 mg

atrazine was administered to rats by gavage, 20% of the dose was

excreted in the feces within 72 hours. The other 80% was

absorbed across the lining of the gastrointestinal tract into the

bloodstream. After 72 hours, 65% was eliminated in the urine and

15% was retained in body tissues, mainly in the liver, kidneys

and lungs (24).

ECOLOGICAL EFFECTS

Effects on Birds

Atrazine is only slightly toxic to birds. The LD50 in

mallard ducks is greater than 2,000 mg/kg. The NOELs for

bobwhite quail and ring-necked pheasants fed atrazine were both

greater than 5,000 ppm.

Effects on Aquatic Organisms

Atrazine is only slightly toxic to fish and other pond or

stream life. In whitefish, atrazine accumulates in the brain,

gall bladder, liver and gut (Arch. Hydrobiol. Suppl.

59(2-3):252-87. 1981). Fish may bioaccumulate atrazine to levels

of 11 times the concentration in surrounding water. This is a

low level of bioaccumulation. Atrazine is easily broken down.

Effects on Other Animals (Nontarget species)

Atrazine is not toxic to bees (25).

ENVIRONMENTAL FATE

Breakdown of the Chemical in Soil and Groundwater

Atrazine is moderately to highly mobile in soils, especially

where soils have low clay or organic matter content. Because it

does not absorb strongly to soil particles (Koc = 100 g/ml) and

it has a lengthy soil half-life (60 to 100+ days), it is expected

to have a high potential for groundwater contamination, even

though it is only moderately soluble in water (33 ug/ml) (26,

29).

Atrazine is not normally found below the first foot of soil,

even after years of continuous use.

Chemical hydrolysis, followed by degradation by soil

microorganisms probably account for most of the breakdown of

atrazine in soil. Hydrolysis is rapid in acidic or basic

environments, but is slower at neutral pHs. Addition of humic

material increased the rate of hydrolysis. Atrazine is also

subject to photo-decomposition and volatilization when high

temperatures and prolonged sunlight occur after precipitation,

but these effects are small under normal field conditions.

Atrazine can persist for longer than one year under conditions

which are not conducive to chemical or biological activity, such

as dry or cold climates (27, 28). Atrazine usually lasts about 4

months at the surface and 2 months at deeper sites

(Agro-Ecosystems 7(3):225238.1981).

Breakdown of the Chemical in Water

Atrazine is not very water soluble. Chemical hydrolysis,

followed by biodegradation, may be the most important route of

disappearance from aquatic environments. Hydrolysis is rapid

under acidic or basic conditions, but is slower at neutral pHs.

Addition of humic material increased the rate of hydrolysis.

Atrazine is not expected to strongly adsorb to sediments.

Bioconcentration and volatilization of atrazine are not

environmentally important (27).

Trace amounts of atrazine have been found in drinking water

samples from Louisiana and Iowa and in groundwater samples from

Pennsylvania, Iowa, Nebraska, Wisconsin and Maryland (27, 29, NRC

Drinking Water and Health 1977). Atrazine has been detected in

each of 146 water samples collected at 8 locations from the

Mississippi, Ohio and Missouri Rivers and their tributaries. For

several weeks, 27% of these samples contained atrazine at

concentrations above the EPA's maximum concentration level (MCL)

for atrazine of 3 ppb. The MCL is the maximum permissible level

of a contaminant in water delivered to any user of a public water

system (30). A five year survey of drinking water wells

detected trace amounts of atrazine in an estimated 1.7% of

community water systems and 0.7% of rural domestic wells

nationwide. Levels detected in rural domestic wells sometimes

exceeded the MCL (31).

Breakdown of the Chemical in Vegetation

Atrazine is absorbed by plants mainly through the roots, but

also through the foliage. Once absorbed, atrazine is

translocated upward and accumulates in the growing tips and the

new leaves of the plant. In susceptible plant species, atrazine

inhibits photosynthesis. In tolerant plants, it is metabolized

(28).

Most crops can be planted one year after application of

atrazine. Atrazine blocks the plant's ability to carry on

photosynthesis (Hartley. Agrochem Hdbk 1983). Atrazine

increases the uptake of arsenic by treated plants (such as

grapes) (7).

PHYSICAL PROPERTIES AND GUIDELINES

Atrazine is a white, crystalline solid (25). It is stable

under normal temperatures and pressures, but may burn if exposed

to heat or flame. Excessive heating of atrazine may cause the

production of toxic and corrosive fumes of chlorides and of toxic

fumes of nitrogen. Atrazine is stable in neutral, slightly

acidic, or basic material, but it is hydrolyzed by alkali or

mineral acids at higher temperatures (24, 33).

Occupational Exposure Limits:

5 mg/m3 OSHA TWA

5 mg/m3 ACGIH TWA

5 mg/m3 NIOSH recommended TWA

2 mg/m3 DFG MAK TWA (total dust)

Physical Properties

CAS #: 1912-24-9

Specific gravity: 1.187 g/cubic cm (7, 33)

H20 solubility: 33 ppm at 25 degrees C (25, 26). 0.007% at 25

degrees C (33)

Solubility in other solvents:

Solvent T (degrees C) Solubility

_______ _____________ ___________

Chloroform 25 52,000 ppm (22)

Diethyl ether 27 1.2% (2)

Dimethyl sulfoxide 27 18.3% (2)

Ether 25 12,000 ppm (22)

Ethyl acetate 27 2.8% (2)

Methanol 25 18,000 ppm (22)

N-pentane 27 360 ppm (2)

Melting point: 173-175 degrees C (25).

Vapor pressure: 3.0 x 10 to the minus 7th power mm Hg at 20

degrees C (2, 28). Atrazine is slightly volatile.

Koc: 100 g/ml (26): 0.6 on sandy loam; 1.8 on gravelly sand; 5.6

on silty clay; 7.9 on clay loam; 8.7 on sandy loam, 11.6 on silty

clay loam; and greater than 21 on peat (29)

Chemical Class/Use: triazine herbicide

BASIC MANUFACTURER

Ciba-Geigy

Agricultural Division

PO Box 18300

Greensboro, NC 27419-8300

Review by Basic Manufacturer:

Comments solicited: January, 1992

Comments received: April, 1992

REFERENCES

(1) Meister, R.T. (ed.) 1987. Farm Chemicals Handbook.

Willoughby, OH: Meister Publishing Co.

(2) WSSA Herbicide Handbook Committee. 1983. Herbicide

Handbook of the Weed Science Society of America. 5th Ed. WSSA,

Champaign, IL.

(3) EPA-SAB-74-001 Herbicide Report Chemical Analysis,

Environmental Effects, Agriculture and Other Applied Uses.

Hazardous Materials Advisory Committee. EPA. May 1974.

(4) Tucker, Richard. 1970. Handbook of toxicity of pesticides

to wildlife. USDI Fish & Wildlife Service.

(5) Worthing, C.R. (ed.). 1987. The pesticide manual: A world

compendium. 8th Ed. The British Crop Protection Council.

Croydon, England.

(6) Hayes, Wayland, Jr. 1982. Pesticides studied in man.

Baltimore, MD: Williams & Wilkins.

(7) Kearney, P.C. & D.D. Kaufman (eds.). 1975. Herbicides:

chemistry, degradation, and mode of action. 2nd Ed. Vol. 1 & 2.

New York: M. Dekker.

(8) Hartley, D. and H. Kidd, (eds.) 1983. The agrochemicals

handbook. Nottingham, England: Royal Society of Chemistry.

(9) Crop Protection Chemicals Reference. 1986. 2nd Ed. New

York: Chemical and Pharmaceutical Pub. Corp.

(10) Shepard, T.H. 1973. Catalog of teratogenic agents.

Baltimore, MD: John Hopkins University Press.

(11) Schardein, James. 1985. Chemically induced birth defects.

New York: Marcel Dekker.

(12) U.S. Department of Health, Education and Welfare. 1976.

Suspected Carcinogens. A subfile of the registry of toxic

effects of chemical substances. Washington, DC: EPA.

(13) Department of Transportation. 1984. Emergency Response

Guidebook: Guidebook for hazardous materials incidents.

Washington, DC: U.S. DOT.

(14) Hallenbeck, W.H. & K.M. Cunningham-Burns. 1985.

Pesticides and human health. New York: Springer-Verlag.

(15) Lef'evre, M.J. 1980. First aid manual for chemical

accidents. New York: Van Nostrand Reinhold.

(16) TOXNET. 1985. National library of medicine's toxicology

data network. Hazardous Substances Databank. Public Health

Service. National Institute of Health. U.S. Department of

Health and Human Services. Bethesda, MD: NLM.

(17) Sax, N.I. 1975. Dangerous properties of industrial

materials. 4th Ed. New York: Van Nostrand Reinhold Co.

(18) Casarett, L.J. 1980. Casarett & Doull's Toxicology: the

basic science of poisons. 2nd Ed. New York: Macmillan.

(19) Gosselin, R.E. 1984. Clinical toxicology of commercial

products. 5th Ed. Baltimore, MD: Williams & Wilkins.

(20) National Fire Protection Association (NFPA). 1978. Fire

Protection Guide. Hazardous Materials.

(21) Morgan, D.P. 1982. Recognition and management of

pesticide poisonings. Iowa Pesticide Hazardous Assessment

Project. 1982. Iowa City, IA.

(22) Windholz, M. (ed.) 1976. The Merck Index: an

encyclopedia of chemicals and drugs. 9th Ed. Rahway, NJ:

Merck.

(23) Sunshine, Irving. 1969. Handbook of analytical

toxicology. Cleveland, OH: Chemical Rubber Co.

(24) Hayes, W.J. and E.R. Laws (ed.). 1990. Handbook of

Pesticide Toxicology, Vol. 3, Classes of Pesticides. Academic

Press, Inc., New York.

(25) Meister, R.T. (ed.). 1992. Farm Chemicals Handbook '92.

Meister Publishing Company, Willoughby, Ohio.

(26) USDA SCS. 1990 (Nov). SCS/ARS/CES Pesticide Properties

Database: Version 2.0 (Summary). USDA - Soil Conservation

Service, Syracuse, NY.

(27) Howard, P.H. (ed.). 1989. Handbook of Environmental Fate

and Exposure Data for Organic Chemicals, Vol. III: Pesticides.

Lewis Publishers, Chelsea, Michigan.

(28) WSSA Herbicide Handbook Committee. Herbicide Handbook of

the Weed Science Society of America, 6th Ed. WSSA, Champaign, IL.

1989.

(29) US EPA. 1988 (August). Atrazine: Health Advisory. Office

of Drinking Water, US EPA, Washington, DC.

(30) USGS. 1991 (Nov. 20). Spring sampling finds herbicides

throughout Mississippi River and tributaries. U.S. Geologic

Survey, Dept. of the Interior, Reston, Virginia.

(31) US EPA. 1990 (Fall). National Pesticide Survey: Atrazine.

Office of Water and Office of Pesticides and Toxic Substances, US

EPA, Washington, DC.

(32) Food Chemical News, Inc. 1990 (Jan. 31). Atrazine use

restricted; other label changes imposed by EPA. Pesticide and

Toxic Chemical News. Washington, DC.

(33) OHS MSDS for Atrazine. 1991 (March 20).

This PIP is part of the EXTOXNET Pesticide Information

Notebook. For more information, contact the Pesticide Management

Education Program, Cornell University, 5123 Comstock Hall,

Ithaca, N.Y. 14853.

DISCLAIMER: The information in this profile does not in any way

replace or supersede the information on the pesticide product

label/ing or other regulatory requirements. Please refer to the

pesticide product label/ing.